Cafe 101 is very well-known among both the Chinese community in Atlanta and the general eating public. It has a Taiwanese spin, which particularly shows up in the desserts, as we will see in a minute.
My favorite dish there is the basil chicken. It's a pretty subtle dish: the basil and some sweetness in the sauce are counterbalanced by heat from peppers and astringency from garlic. As you can see, it's served in a hot pot, so you get some sizzling action as well. I've never seen this anywhere else and I really enjoy it.
Although I didn't get dessert today, I've had their desserts on many occasions. This is where the Taiwanese spin is most visible. Taiwan, because of its warm climate, has wonderful fruits of all varieties. Cafe 101's desserts combine various fruit slices with shaved ice, tapioca, and condensed milk. It's extremely refreshing and should be healthier than your average dessert.